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Although there is some useful autobiographical material including diaries and family correspondence among the papers, the bulk of the material relates to Broad's working life. The detailed faculty lectures, many of which were later published, are preserved as are other lectures that Broad gave from time to time. Notes of the works of others are also among the papers, with Broad's comments, but little of Broad's own notes in preparation for his lectures and publications survive. There are also eight undated notebooks on subjects related to psychical research. Additionally, there are a few classical papers of Arthur Verrall, which Broad was presumably given due to the SPR connection with the family and some papers of John Chadwick on mathematical and philosophical subjects

Papers relating to psychical research and other occult subjects, the Perrott Fellowship, the Arthur Stanley Eddington Memorial Lecture, and the Swedish language, with group photographs relating to Dulwich College.