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The papers consist of correspondence, diaries, subject files, writings, other Whewell papers, family papers, and later papers of others. The family papers include those originally gathered by Whewell's first wife Cordelia (née Marshall) and his second wife Lady Affleck (née Ellis). The papers of Lady Affleck's brother and Whewell's friend Robert Leslie Ellis now form a subset of this collection. The collection is further described in the System of arrangement field below, and materials received by gift and by purchase are described in the Related units of description field below.

Sixty-six lectures on constitutional history written in Winstanley's hand on loose sheets of paper, each headed with a lecture number and title, accompanied by a holograph book list relating to study of the 16th century and an incomplete lecture/review? on George I and his relationship with his Cabinet and Secretaries of State. The items are undated but presumably date from one of Winstanley's tenures at Cambridge, i.e. 1906-14 and 1919-35.

The archive includes diaries 1952-59, records of self-analysis 1939-59, correspondence 1925-1980s, student notes of G E Moore's lectures 1923-24, academic papers (many fragmentary) ?1920s-1980s

The largest surviving portion of Wittgenstein's nachlass containing his working papers 1914-1951