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The majority of this archive consists of letters by Duff to members of his family, viz.: (A): to his wife Laura, 45 letters, 1897-1909; (B): to his son Alan, 356 letters, 1909-1933; (C): to his son Patrick, 96 letters, 1909-1934; (D): to his son James, 4 letters, 1909-1916; (E): to his daughter Hester, 8 letters, 1933-1934; (F): to his daughter Mary, 1 letter, 1911.

There are also 68 letters (G) from Laura Duff to her son Alan, 1915-1940, and three (H) to her husband J.D. Duff, relating to their son James's entrance examinations for Wellington College in 1910. J, K and L are letters written by their sons: 3 letters and a postcard from Alan Duff to his mother, 1909-1920 (J), a letter from James Duff to Alan Duff, 1911 (K), and a letter from Patrick Duff to J. F. Duff, relating to J. F. Duff winning a scholarship to Trinity in 1916 (L).

The final group of letters (M) are by various authors: one from J. D. Duff to Diana Frances Crawley, future wife of his son Alan, on the death of her father, 1933; letters to A. C. Duff from W. G. Collett (1911) and R. Moore (1913) at Wellington College; letter to J. D. Duff from G. M. Trevelyan, 1934 about Edward Fitzgerald's letters; letter to Laura Duff from the Postmaster at Cambridge, 1923, relating to a telegram from Cairo.

Miscellaneous material (N) comprises: copy of the marriage certificate of James Duff Duff and Laura Lenox-Coningham, 1895; page torn from a notebook with short phrase in Ancient Greek; memoir, "Lemnos" of an army camp, probably by A. C. Duff, with envelope addressed to J. D. Duff.

Finally there are twenty eight of J. D. Duff's pocket diaries (usually by Lett's) dating from 1888-1912, 1915-1918, 1922-1926, and 1931-1934; the earliest are kept as appointment books, with brief notes of college and social occasions, but Duff's entries later expand to be fuller records of his days, typically recording weather, reading material, pastimes and family news. A notebook with A. C. Duff's name and address at the front contains 'Extracts from F[ather's] Diary'.

The papers consist of correspondence, printed material, writings, personal papers, and photographs documenting the English life of Erskine Childers. The correspondence includes incoming letters to Erskine and to Molly Childers, copies of letters sent by Erskine, and a large number of letters written to others from others.

There are over 75 letters from Erskine to Molly dated 1903-1913; Erskine's other principal correspondents include Ian Hamilton, Field Marshal Frederick Roberts, and Basil Williams. Molly's principal correspondents include Benoît-Constant Coquelin, Kate Courtney, and John Singer Sargent. The collection includes letters from a variety of other correspondents, among them Edward Arnold, Julian Corbett, Arthur Conan Doyle, Henry James, William James, Lord Kitchener, J. Ellis McTaggart, Walter Runciman, George Bernard Shaw (to Emily Ford), and G. M. Trevelyan.

Printed material includes cuttings of reviews for 'The H.A.C. in South Africa', 'The Times History of the war in South Africa', 'War and the Arme Blanche', 'The Riddle of the Sands', and 'The German Influence on British Cavalry'; cuttings of articles on cruising printed in 'The Times' from 1907-1913; as well as two issues of 'Poblacht na hÉireann' from 21, 23 October, 1922.

The collection also includes a holograph poem apiece by Bronson Alcott and William Ellery Channing, photographs of Benoît-Constant Coquelin, and a signed photograph of Sarah Bernhardt.